Time- and frequency-domain 3-wave mixing spectroscopy is developed as a surface-selective nonlinear technique capable of measuring spectral evolution of vibrational coherences. Hydrogen bond dynamics of interfacial water is observed to proceed on 100 fs timescale.
Femtosecond hydrogen bond dynamics by spectrally- and time-resolved vibrational sum frequency generation
2005 Quantum Electronics and Laser Science Conference ; 3 ; 1884-1886 vol. 3
01.01.2005
1155348 byte
Aufsatz (Konferenz)
Elektronische Ressource
Englisch